Place all ingredients except the pineapple in a mixing bowl and whisk until well combined.
Stir about a cup of the crushed pineapple with juice, reserving the other cup for later use. Pour the pineapple-coconut mixture into popsicle molds, filling each 2/3-3/4 full.
Spoon the remaining cup of crushed pineapple and juice evenly into each mold, on top of the coconut-pineapple mixture, filling to the top.
Insert popsicle sticks and freeze for several hours or overnight.